“…In general, Pr 3+ ions embrace the abundant energy level structure, which is regarded as potential activating ions in various gain materials for visible laser. 6 With the development of blue laser diodes (LDs) and frequency-doubled optically pumped semiconductor laser (2ω-OPLS), high efficiency laser output has been achieved in Pr 3+ ions-doped crystals, such as LiYF 4 (YLF), 7,8 BaY 2 F 8 (BYF), 9 KY 3 F 10 (KYF), 10 LiY 0.3 Lu 0.7 F 4 (LY 0.3 L 0.7 -LF), 11 CaF 2 12 and SrF 2 . 13 In addition, in oxide matrixes, e.g., SrAl 12 O 19 (SRA), 14 YAlO 3 (YAP), 15 and LaMgAl 11 O 19 (LMA), 16 the laser output has also been also realized.…”