Construction
of anisotropic micro-channels in aerogel-based evaporators
has been considered as a promising way to solve the salt accumulation
and contaminant influence issues in the solar-driven interfacial evaporation
process, however, which still suffer from drawbacks like costly fabrications.
Herein, composite aerogels with anisotropic micro-channels were constructed
through a simple co-assembly strategy between biomass chitosan and
WS2 nanosheets. Ascribing to the synergetic effects of
photothermal conversion capabilities of WS2 nanosheets
and hydrophilia of chitosan, as well as the oriented microporous channels
throughout the aerogels, the obtained aerogels (CS/WS2)
exhibited a max evaporation rate of ∼2.10 kg m–2 h–1 and a conversion efficiency of ∼87.9%
under 1 sun illumination and presented continuous production of clean
water even in acidic, alkaline, and organic dye solutions and high-salinity
brines. Thus, this study paves a novel and simple strategy to build
anisotropic micro-channels in aerogel evaporators for efficient and
sustainable solar evaporation and desalination.