Highly reversible aqueous zinc-ion battery using the chelating agent triethanolamine as an electrolyte additive

Lin, Yuehe; Hu, Youzuo; Zhang, Shu; Xu, Ziqiang; Feng, Tingting; Zhou, Haiping; Wu, Mengqiang

doi:10.1039/d2ce01089e

CrystEngComm

2022

DOI: 10.1039/d2ce01089e

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Highly reversible aqueous zinc-ion battery using the chelating agent triethanolamine as an electrolyte additive

Yuehe Lin

Youzuo Hu

Shu Zhang

et al.

Abstract: Aqueous zinc-ion batteries (AZIBs) have been received large attentions owing to the increasing demand for safety and inexpensive batteries. However, poor cycling issue hinders its commercialization and further application, which...

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2024

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Cited by 7 publications

References 56 publications

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A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries

Ren,

Xu,

Chen

et al. 2024

Small

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Na3V2(PO4)3(NVP), as a representative sodium superionic conductor with a stable polyanion framework, is considered a cathode candidate for aqueous zinc‐ion batteries attributed to their high discharge platform and open 3D structure. Nevertheless, the structural stability of NVP and the cathode‐electrolyte interphase (CEI) layer formed on NVP can be deteriorated by the aqueous electrolyte to a certain extent, which will result in slow Zn2+ migration. To solve these problems, doping Si elements to NVP and adding sodium acetate (NaAc) to the electrolyte are utilized as a synergistic regulation route to enable a highly stable CEI with rapid Zn2+ migration. In this regard, Ac− competitively takes part in the solvation structure of Zn2+ in aqueous electrolyte, weakening the interaction between water and Zn2+, and meanwhile a highly stable CEI is formed to avoid structural damage and enable rapid Zn2+ migration. The NVPS/C@rGO electrode exhibits a notable capacity of 115.5 mAh g−1 at a current density of 50 mA g−1 in the mixed electrolyte (3 M ZnOTF2+3 M NaAc). Eventually, a collapsible “sandwich” soft pack battery is designed and fabricated and can be used to power small fans and LEDs, which proves the practical application of aqueous zinc‐ion batteries in flexible batteries.

show abstract

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries

Ren,

Xu,

Chen

et al. 2024

Small

View full text Add to dashboard Cite

show abstract

Stabilizing Zn anode for high-performance Zn-Ni battery through a complexing agent electrolyte addition

Liang,

Wu,

Wang

et al. 2024

Journal of Colloid and Interface Science

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Stabilization of cathode electrolyte interphase for aqueous zinc-ion batteries

Yao,

Zhang,

Zhu

2024

Journal of Energy Chemistry

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Highly reversible aqueous zinc-ion battery using the chelating agent triethanolamine as an electrolyte additive

Abstract: Aqueous zinc-ion batteries (AZIBs) have been received large attentions owing to the increasing demand for safety and inexpensive batteries. However, poor cycling issue hinders its commercialization and further application, which...

Cited by 7 publications

References 56 publications

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries

Stabilizing Zn anode for high-performance Zn-Ni battery through a complexing agent electrolyte addition

Stabilization of cathode electrolyte interphase for aqueous zinc-ion batteries

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Highly reversible aqueous zinc-ion battery using the chelating agent triethanolamine as an electrolyte additive

Abstract: Aqueous zinc-ion batteries (AZIBs) have been received large attentions owing to the increasing demand for safety and inexpensive batteries. However, poor cycling issue hinders its commercialization and further application, which...

Cited by 7 publications

References 56 publications

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn2+ Migration Toward Advanced Flexible Zinc‐Ion Batteries

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn2+ Migration Toward Advanced Flexible Zinc‐Ion Batteries

Stabilizing Zn anode for high-performance Zn-Ni battery through a complexing agent electrolyte addition

Stabilization of cathode electrolyte interphase for aqueous zinc-ion batteries

Contact Info

Product

Resources

About

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries

A Synergistically Regulated Cathode/Electrolyte Interphase With High Stability and Rapid Zn²⁺ Migration Toward Advanced Flexible Zinc‐Ion Batteries