2023
DOI: 10.1038/s41467-023-36714-7
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Hybrid molecular graphene transistor as an operando and optoelectronic platform

Abstract: Lack of reproducibility hampers molecular devices integration into large-scale circuits. Thus, incorporating operando characterization can facilitate the understanding of multiple features producing disparities in different devices. In this work, we report the realization of hybrid molecular graphene field effect transistors (m-GFETs) based on 11-(Ferrocenyl)undecanethiol (FcC11SH) micro self-assembled monolayers (μSAMs) and high-quality graphene (Gr) in a back-gated configuration. On the one hand, Gr enables … Show more

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Cited by 9 publications
(7 citation statements)
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“…The challenges to engineering good electrical contact to graphene surfaces in molecular electronics are recognised, and future generations of this design strategy which enhance molecule–graphene coupling at the top electrode interface are being explored. 91–93…”
Section: Resultsmentioning
confidence: 99%
“…The challenges to engineering good electrical contact to graphene surfaces in molecular electronics are recognised, and future generations of this design strategy which enhance molecule–graphene coupling at the top electrode interface are being explored. 91–93…”
Section: Resultsmentioning
confidence: 99%
“…Overall, this field of long-chain molecules that are able to perform logic operations seems to be underdeveloped, with few examples (see also References [25][26][27][28][29]). Nevertheless, the possibility of synthesizing such macromolecules with tailor-made characteristics appears quite attractive.…”
Section: Long-chain Molecules As Logic Gates (Lc-mlg)mentioning
confidence: 99%
“…The use of the anthracene moiety as a fluorophore has long been realized in the realm of ferrocene-based MLGs, although its implementation has not been that successful compared to naphthalimide. This can be rationalized based on the synthetic difficulties of Overall, this field of long-chain molecules that are able to perform logic operations seems to be underdeveloped, with few examples (see also References [25][26][27][28][29]). Nevertheless, the possibility of synthesizing such macromolecules with tailor-made characteristics appears quite attractive.…”
Section: Imentioning
confidence: 99%
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