Hydrodeoxygenation of lignin bio-oil model compounds and surrogate mixtures over zeolite supported nickel catalysts

Zormpa, Foteini F.; Margellou, Antigoni G.; Karakoulia, Stamatia A.; Delli, Evangelia; Triantafyllidis, Konstantinos S.

doi:10.1016/j.cattod.2024.114654

Catalysis Today

2024

DOI: 10.1016/j.cattod.2024.114654

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Hydrodeoxygenation of lignin bio-oil model compounds and surrogate mixtures over zeolite supported nickel catalysts

Foteini F. Zormpa,

Antigoni G. Margellou,

Stamatia A. Karakoulia

et al.

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2024

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Cited by 3 publications

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Sustainable Liquid‐Organic‐Hydrogen‐Carrier‐Based Hydrogen‐Storage Technology Using Crude or Waste Feedstock/Hydrogen

Kim,

Yoon,

Kim

et al. 2024

Adv Energy and Sustain Res

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For liquid organic hydrogen carrier (LOHC) technology to be competitive with other H2‐storage methods, it is crucial to reduce the cost of LOHC materials occupying the high proportion of the embodied energy required for system implementation. Promising approaches are to convert crude or waste feedstock into LOHC materials and to utilize crude hydrogen sources obtained from various routes. Thus, in this review, the state‐of‐the‐art advances in sustainable LOHC‐based hydrogen storage using crude or waste feedstock, associated with their conversion into LOHC materials, and coupling crude hydrogen with LOHC system to obtain high‐purity H2 without separation and purification are highlighted. Petroleum sources like light cycle oil and pyrolysis fuel oil are used after liquid–liquid extraction, combined distillation/hydroprocessing, and one‐pot hydrotreating–hydrocracking. In case of converting renewable resources (e.g., biomass and plastic waste), depolymerization followed by hydrodeoxygenation is an effective approach. To utilize crude hydrogen sources for hydrogen storage, catalysts should be designed and synthesized toward activating LOHC hydrogenation reaction at lower temperatures, along with high CO resistance. Consequently, this context provides guidance for the development of LOHC technology to accelerate its commercialization.

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Sustainable Liquid‐Organic‐Hydrogen‐Carrier‐Based Hydrogen‐Storage Technology Using Crude or Waste Feedstock/Hydrogen

Kim,

Yoon,

Kim

et al. 2024

Adv Energy and Sustain Res

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Conversion of beechwood organosolv lignin via fast pyrolysis and in situ catalytic upgrading towards aromatic and phenolic-rich bio-oil

Soldatos,

Margellou,

Pappa

et al. 2024

Sustainable Chemistry for the Environment

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Efficient Production of Platform Chemicals from Lignocellulosic Biomass by Using Nanocatalysts: A Review

Jain,

Kassaye

2024

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This paper discusses significant advancements in using lignocellulosic biomass for the sustainable production of biofuels and chemicals. As fossil-based resources decline and environmental concerns rise, the paper emphasizes the role of integrated biorefineries in producing renewable liquid fuels and high-value chemicals from biomass. It highlights exploring various green pathways for biomass conversion, with a particular focus on nanocatalysis. Due to their large surface area-to-volume ratio, nanocatalysts provide enhanced catalytic activity and efficiency in biomass transformation processes. The review delves into the synthesis of value-added and furfural platform chemicals alongside the hydrogenolysis of 5-hydroxymethylfurfural (5-HMF) into biofuels like 2,5-dimethylfuran (DMF) and 2,5-dimethyltetrahydrofuran (DMTHF). The paper ultimately underscores the importance of nanotechnology in achieving high yield and selectivity in the biomass conversion process, positioning it as a promising approach for future sustainable energy and chemical production.

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Hydrodeoxygenation of lignin bio-oil model compounds and surrogate mixtures over zeolite supported nickel catalysts

Cited by 3 publications

References 91 publications

Sustainable Liquid‐Organic‐Hydrogen‐Carrier‐Based Hydrogen‐Storage Technology Using Crude or Waste Feedstock/Hydrogen

Sustainable Liquid‐Organic‐Hydrogen‐Carrier‐Based Hydrogen‐Storage Technology Using Crude or Waste Feedstock/Hydrogen

Conversion of beechwood organosolv lignin via fast pyrolysis and in situ catalytic upgrading towards aromatic and phenolic-rich bio-oil

Efficient Production of Platform Chemicals from Lignocellulosic Biomass by Using Nanocatalysts: A Review

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