In this study, we
conduct simulation research on simultaneous desulfurization
and denitrification in a multistaggered baffle spray scrubber. By
employing two-phase flow simulations within the Euler–Lagrange
framework and calculating the gas–liquid mass transfer rate
with user-defined functions, we comprehensively analyzed the effects
of various operational parameters. Initially, we validated our simulation
model by comparing the simulation results with experimental data.
Under conditions of a 0.2 mm droplet diameter, a liquid-to-gas ratio
(L/G) of 12 L/m3, and a gas flow rate of 5 CMM using a
full cone nozzle, the simulation indicated a desulfurization efficiency
of 99.90 versus 99.84% obtained experimentally and a denitrification
efficiency of 92.01 versus 90.67% obtained experimentally. This comparison
confirmed the reliability of the simulation model. Our findings indicate
that a droplet size of 2 mm is optimal, enhancing the desulfurization
efficiency from 99.90 to 99.98% and the denitrification efficiency
from 92.01 to 99.76%. However, when the droplet size exceeds 2 mm,
efficiencies marginally decrease. Increasing the liquid-to-gas ratio
to 16 L/m3 further improves desulfurization and denitrification
efficiencies to 99.98 and 99.80%, respectively. In contrast, higher
inlet flue gas flow rates reduce these efficiencies, with a decline
observed from 100% to as low as 93.90% for denitrification with 2
mm droplets. Additionally, the use of a swirl cone nozzle, compared
to full or hollow cone nozzles, better disperses droplets, enhancing
the gas–liquid contact and achieving efficiencies of 99.99%
for desulfurization and 99.81% for denitrification with 2 mm droplets.
These insights are valuable for optimizing operational conditions
in industrial-scale spray scrubbers, significantly contributing to
mitigating the environmental impacts of industrial emissions.