Carbon
capture and storage (CCS) technology has been widely investigated
to decrease the greenhouse effect. Geological CO2 storage
sites are targeted mainly on depleted petroleum reservoirs or deep
saline aquifers. However, CO2 leakage might take place
through wellbores, cap rocks, reservoir fractures, or faults during
or after the process of CO2 storage leading to environmental
problems. To minimize these hazards, different kinds of sealants have
been developed and applied. This review aims to summarize those materials
applicable to CO2 leakage remediation. On the basis of
the sealing mechanisms and compositions of different sealant materials,
they were divided into seven major types: Portland cement, geopolymer
cement, resins, biofilms barriers, gel systems, foams, and nanoparticles.
For different types of sealants, their application background, chemical
and physical properties, CO2 leakage remediation mechanism,
impact factors of sealing performance, advantages, and limitations
were summarized. Future development directions for these sealant materials
are also recommended. To solve the problem caused by the weak acid-resistant
performance of Portland cement, anti-CO2 materials should
be developed and added to the formulation. Environmentally friendly
materials need to be designed to replace some current user-hostile
compositions in the geopolymer cement. Moreover, chemicals that can
control the geopolymerization process are also required because of
the high curing temperature requirement for the recent geopolymer
productions. The injectivity of Portland cement and resin limits its
application for in-depth CO2 leakage control; however,
gels with relatively low viscosity during the injection can be a good
alternative, although their thermal stability and strength need to
be further enhanced. Biotechnology and nanotechnology are perspectives
to be applied in the CO2 leakage control process. Foams
with good stability might be used for CO2 leakage remediation
in the porous medium without fractures, but their life cycle should
be prolonged.