During oil and gas well construction, lost circulation
caused substantial
nonoperation time and extra costs, and hydrogel, resilient and environmentally
friendly, was one of the major types of material for lost circulation
treatment. To migrate the weak bonding and hydrothermal degradation
of conventional single network hydrogels, dual network (DN) hydrogel
was prepared and immersed in solvents of polyethylene glycol (PEG),
ethylene glycol, and glycerol. The swelling of DN gels at different
temperatures was studied with water content and swelling rate tests,
and the gel structural and morphology was characterized with attenuated
total reflectance infrared spectroscopy (ATR-IR) and scanning electron
microscopy test. Then, the compression test and fracture plugging
performance test were conducted to study the strength of the gel.
The results show that compared to those in ethylene glycol and glycerin,
DN gel after immersion in PEG (DN-PEG) exhibits greater compression
strength and better plugging performance even at high temperatures.
The compression strength of DN-PEG was twice that of DN hydrogel before
immersion, and its fracture plug breaking pressure can reach over
10.0 MPa. After undergoing hydrothermal treatment at 90 °C, the
compression strength of the DN-PEG was nearly 20 times that of the
DN hydrogel, and the fracture plug breaking pressure was still 2.81
MPa. According to ATR-IR spectroscopy, as the molecular weight of
the solvent increases, more hydroxyl groups in the PEG have better
ability to bind with hydrogen bonds, which greatly inhibits the swelling
and polymer chain breakage, thereby reducing hydrothermal degradation
in the strength of the dual-network hydrogel. Our work proposed an
effective method to reduce the degradation of hydrogel in water at
high temperature, and the prepared DN-PEG hydrogel was a promising
material for lost circulation treatments in fractured formation.