Abstract. The Indo-Gangetic Plain (IGP) experienced an intensive air
pollution episode during November 2017. Weather Research and Forecasting
model coupled to Chemistry (WRF-Chem), a coupled meteorology–chemistry model, was
used to simulate this episode. In order to capture PM2.5 peaks, we
modified input chemical boundary conditions and biomass burning emissions.
The Community Atmosphere Model with Chemistry (CAM-chem) and Modern-Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) global models provided gaseous and aerosol chemical
boundary conditions, respectively. We also incorporated Visible Infrared
Imaging Radiometer Suite (VIIRS) active fire
points to fill in missing fire emissions in the Fire INventory from NCAR (FINN) and scaled by a factor of
7 for an 8 d period. Evaluations against various observations
indicated the model captured the temporal trend very well although missed
the peaks on 7, 8, and 10 November. Modeled aerosol
composition in Delhi showed secondary inorganic aerosols (SIAs) and secondary
organic aerosols (SOAs) comprised 30 % and 27 % of total PM2.5 concentration, respectively, during November, with a modeled OC/BC ratio
of 2.72. Back trajectories showed agricultural fires in Punjab were the
major source for extremely polluted days in Delhi. Furthermore, high
concentrations above the boundary layers in vertical profiles suggested
either the plume rise in the model released the emissions too high or the
model did not mix the smoke down fast enough. Results also showed long-range-transported dust did not affect Delhi's air quality during the episode.
Spatial plots showed averaged aerosol optical depth (AOD) of 0.58 (±0.4) over November. The model AODs were biased high over central India and
low over the eastern IGP, indicating improving emissions in the eastern IGP can
significantly improve the air quality predictions. We also found high ozone
concentrations over the domain, which indicates ozone should be considered
in future air quality management strategies alongside particulate matter.