2023
DOI: 10.1021/acs.nanolett.3c01463
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Impact of Plasmonic and Dielectric Substrates on the Whispering-Gallery Modes in Self-Assembled Fluorescent Semiconductor Polymer Microspheres

Abstract: In this work, the impact of metallic and dielectric conducting substrates, gold and indium tin oxide (ITO)-coated glass, on the whispering gallery modes (WGMs) of semiconductor π-conjugated polymer microspheres is investigated. Hyperspectral mapping was performed to obtain the excitation-position-dependent emission spectra of the microspheres. Substrate-dependent quenching of WGMs sensitive to mode polarization was observed and explained. On a glass substrate, both transverse-electric (TE) and transverse-magn… Show more

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Cited by 3 publications
(1 citation statement)
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“…Because WGMs are circularly con ned modes at the sphere surface, they are highly sensitive to the surface molecular arrangement. 35 In this article, we demonstrate distinct impacts on WGM resonance arising from topological textures formed on a spherical microcavity. Mechanically and optically robust microspheres with a TB topology are prepared by a self-assembly process in solution.…”
Section: Introductionmentioning
confidence: 81%
“…Because WGMs are circularly con ned modes at the sphere surface, they are highly sensitive to the surface molecular arrangement. 35 In this article, we demonstrate distinct impacts on WGM resonance arising from topological textures formed on a spherical microcavity. Mechanically and optically robust microspheres with a TB topology are prepared by a self-assembly process in solution.…”
Section: Introductionmentioning
confidence: 81%