Frequency conversion of nonclassical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic linear-optics approach to spectral shearing of quantum light pulses and show it preserves the wavepacket coherence and quantum nature of light. The technique is based upon an electro-optic Doppler shift to implement frequency shear of heralded single-photon wave packets by ±200 GHz, which can be scaled to an arbitrary shift. These results demonstrate a reconfigurable method to controlling the spectral-temporal mode structure of quantum light that could achieve unitary operation.The frequency of a single light quantum, or photon, is a key physical property of individual excitations of the quantized electromagnetic field [1], which were introduced to describe the photoelectric effect [2]. Frequency is a mode characteristic, just as polarization, transverse-spatial amplitude, and direction of propagation define the modes of electromagnetic radiation. Thus frequency can be transformed using linear-optical elements in much the same way lenses transform transverse-spatial modes and wave plates manipulate polarization modes. Frequency is not an immutable property of photons-it can be coherently and deterministically modified. For example, retroreflection from a moving mirror results in a frequency shift due to the Doppler effect [3,4]. The various independent degrees of freedom that comprise the modes of light can be used to encode information in the electromagnetic field, namely position-momentum, time-frequency, and polarization. Information-technology applications require precise means for manipulation and measurement of light in the encoding degree of freedom. Many preliminary demonstrations of quantum optical technologies have utilized polarization, path or transverse-spatial mode encoding. These degrees of freedom are limited to relatively few quantum bits that can be practically addressed per photon within an integrated-optics platform, in which high-stability, low-loss multiphoton interference, necessary for optical quantum technologies, can occur. Recently, the time-frequency (TF) mode structure of light has come to the fore in quantum photonics as an ideal means of quantum information encoding for integrated optical quantum technologies [5][6][7][8][9][10][11].Essential to both quantum and classical technologies based upon TF mode encoding is the ability to control the pulsemode structure of light-where the central frequency and arrival time play prominent roles. In the classical domain the primary methods to control an optical pulse are based upon direct modification of the wave packet by amplifying and filtering different frequency and time components [12,13]. This approach to pulse shaping is incompatible with quantum states of light owing to noise and signal degradation arising from amplification and loss, resulting in destruction of the fragile quantum coherences between di...