The enhancement of double strengthening by nanoparticles and nanoscale precipitates in diecast Al-Si-Mg-Mn-TiB2 composites has be achieved by introducing TiB2 nanoparticles into Al-*Si-*Mg alloy fabricated by super vacuum assisted high pressure die casting process. The composite with 3.5wt.% TiB2 nanoparticles could deliver the hardness of 1.5 GPa, the yield strength of 351 MPa and ultimate tensile strength of 410 MPa in association with an industrially applicable ductility of 5.2 %, after solution and peak ageing heat treatment. The TiB2 nanoparticles distributed at the grain boundaries rather than in the α-Al matrix of the composites in as-cast state. After solution and peak ageing, the TiB2 nanoparticles were enrolled into the α-Al matrix through the combining and coarsening of the α-Al phase during heat treatment, and nanoscale β′′ precipitates formed in the α-Al matrix. Both the TiB2 nanoparticles and the nanoscale β′′ precipitates had highly coherent interfaces with the α-Al matrix, i.e., Al(11-1)//TiB2(0001), Al[011]//TiB2[11-20], Al[320]//β''(a-axis), Al[1-30]//β''(caxis) and Al(020)//β''(b-axis), confirming strong interfacial strengthening. The double strengthening of the TiB2 nanoparticles and the nanoscale β′′ precipitates dispersing in the α-Al matrix resulted in the milestone high strength of the composites.