In situ studies of ion irradiated inverse spinel compound magnesium stannate (Mg2SnO4)

Xu, Peng; Tang, Ming; Nino, Juan C.

doi:10.1016/j.jnucmat.2009.02.019

Journal of Nuclear Materials

2009

DOI: 10.1016/j.jnucmat.2009.02.019

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In situ studies of ion irradiated inverse spinel compound magnesium stannate (Mg2SnO4)

Peng Xu

Ming Tang

Juan C. Nino

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Cited by 8 publications

(1 citation statement)

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“… 34 ) and Mg 2 SnO 4 (ref. 35 ). These studies see significant differences in the radiation damage response of spinels as a function of chemistry.…”

mentioning

confidence: 99%

Opposite correlations between cation disordering and amorphization resistance in spinels versus pyrochlores

Uberuaga

Tang

Jiang³

et al. 2015

Nat Commun

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Understanding and predicting radiation damage evolution in complex materials is crucial for developing next-generation nuclear energy sources. Here, using a combination of ion beam irradiation, transmission electron microscopy and X-ray diffraction, we show that, contrary to the behaviour observed in pyrochlores, the amorphization resistance of spinel compounds correlates directly with the energy to disorder the structure. Using a combination of atomistic simulation techniques, we ascribe this behaviour to structural defects on the cation sublattice that are present in spinel but not in pyrochlore. Specifically, because of these structural defects, there are kinetic pathways for the relaxation of disorder in spinel that are absent in pyrochlore. This leads to a direct correlation between amorphization resistance and disordering energetics in spinel, the opposite of that observed in pyrochlores. These results provide new insight into the origins of amorphization resistance in complex oxides beyond fluorite derivatives.

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“… 34 ) and Mg 2 SnO 4 (ref. 35 ). These studies see significant differences in the radiation damage response of spinels as a function of chemistry.…”

mentioning

confidence: 99%

Opposite correlations between cation disordering and amorphization resistance in spinels versus pyrochlores

Uberuaga

Tang

Jiang³

et al. 2015

Nat Commun

View full text Add to dashboard Cite

show abstract

Synthesis and colour properties of pigments based on terbium-dopped Mg2SnO4

Dohnalová

Šulcová

Trojan

2010

J Therm Anal Calorim

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Mechanically assisted solid state synthesis of Mg2SnO4

Berbenni

Milanese

Bruni

et al. 2011

J Therm Anal Calorim

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In situ studies of ion irradiated inverse spinel compound magnesium stannate (Mg2SnO4)

Cited by 8 publications

References 44 publications

Opposite correlations between cation disordering and amorphization resistance in spinels versus pyrochlores

Opposite correlations between cation disordering and amorphization resistance in spinels versus pyrochlores

Synthesis and colour properties of pigments based on terbium-dopped Mg2SnO4

Mechanically assisted solid state synthesis of Mg2SnO4

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