“…The second explanation is that Bi reduces the additional energy barrier at the step edge of islands E a : The reduced E a lowers the probability of nucleation on top of the island even if the island density does not change by the surfactant, leading to layer-by-layer growth. The reduced E a can be caused by either a decrease of E b or by an increase of E d : According to H. A. van der Vegt et al [15], the former is the case for the growth of Cu(1 0 0) [15] and Cu(1 1 1) [16] with In, and the latter which is local effect at the step edge is the case for the growth of Ag(1 1 1) with Sb [17][18][19]. When we deposited Bi on the Fe(1 0 0)-c(2 Â 2)O surface the RHEED intensities always decreased (not shown), whether the substrate temperature was 100 C or room temperature.…”