Geologic carbon storage is required for achieving negative CO 2 emissions to deal with the climate crisis. The classical concept of CO 2 storage consists in injecting CO 2 in geological formations at depths greater than 800 m, where CO 2 becomes a dense fluid, minimizing storage volume. Yet CO 2 has a density lower than the resident brine and tends to float, challenging the widespread deployment of geologic carbon storage. Here, we propose for the first time to store CO 2 in supercritical reservoirs to reduce the buoyancy-driven leakage risk. Supercritical reservoirs are found at drilling-reachable depth in volcanic areas, where high pressure (p > 21.8 MPa) and temperature (T > 374°C) imply CO 2 is denser than water. We estimate that a CO 2 storage capacity in the range of 50-500 Mt yr −1 could be achieved for every 100 injection wells. Carbon storage in supercritical reservoirs is an appealing alternative to the traditional approach. Plain Language Summary Geologic carbon storage, which consists in returning carbon deep underground, should be part of the solution to effectively reach carbon neutrality by the middle of the century to mitigate climate change. CO 2 has been traditionally proposed to be stored in sedimentary rock at depths below 800 m, where CO 2 becomes a dense fluid, minimizing the required storage volume. Nevertheless, CO 2 is lighter than brine in the traditional concept, so a rock with sufficient sealing capacity should be present above the storage formation to prevent leakage. Indeed, one of the main hurdles to deploy geologic carbon storage is the risk of CO 2 leakage. To reduce this risk, we propose a novel storage concept that consists in injecting CO 2 in reservoirs where the pore water stays in supercritical conditions (pressure and temperature higher than 21.8 MPa and 374°C, respectively) because at these conditions, CO 2 becomes denser than water. Consequently, CO 2 sinks, leading to a safe long-term storage. This concept, which could store a significant portion of the total requirements to decarbonize the economy, should start being implemented in deep volcanic areas, given that supercritical reservoirs are found at relatively shallow depths between 3 and 5 km.