The microstructure of the Al1.0Cr1.4Pr1.6Zr (mass%) alloy after homogenized at 500°C for 400 h has been investigated. Addition of Cr, Pr and Zr in combination into pure aluminum results in the formation of submicron Zr-containing PrCr 2 Al 20 and nanoscale Cr, Pr-containing Al 3 Zr dispersed phases. Compared with the Al1.0Cr1.4Pr and Al1.6Zr alloys, a denser distribution of new fine multicomponent dispersed phases and their superimposition effect are associated with enhanced precipitation-hardening behavior of Al1.0Cr1.4Pr1.6Zr alloy.