We report experimental evidence of a remarkable spontaneous time reversal symmetry breaking in two dimensional electron systems formed by atomically confined doping of phosphorus (P) atoms inside bulk crystalline silicon (Si) and germanium (Ge). Weak localization corrections to the conductivity and the universal conductance fluctuations were both found to decrease rapidly with decreasing doping in the Si:P and Ge:P δ−layers, suggesting an effect driven by Coulomb interactions. In-plane magnetotransport measurements indicate the presence of intrinsic local spin fluctuations at low doping, providing a microscopic mechanism for spontaneous lifting of the time reversal symmetry. Our experiments suggest the emergence of a new many-body quantum state when two dimensional electrons are confined to narrow half-filled impurity bands.Invariance to time reversal is among the most fundamental and robust symmetries of nonmagnetic quantum systems. Its violation often leads to new and exotic phenomena, particularly in two dimensions (2D), such as the quantized Hall conductance in semiconductor heterostructures [1], the quantum anomalous Hall effect in topological insulators [2] or the predicted chiral superconductivity in graphene [3]. The breaking of time reversal invariance is experimentally achieved either by an external magnetic field or intentional magnetic doping. Here we show that strong Coulomb interactions can also lift the time reversal symmetry in nonmagnetic 2D systems at zero magnetic field.While bulk P-doped Si and Ge have been extensively studied in the context of electron localization in three dimensions [4][5][6][7][8][9], confining the dopants to one or few atomic planes (δ−layers) of the host semiconductor has recently led to a new class of 2D electron system [10][11][12][13]. Electron transport in these atomically confined 2D layers occurs within a 2D impurity band where the effective Coulomb interaction is parameterized in terms of U/γ, with U being the Coulomb energy required to add an additional electron to a dopant site, and γ, the hopping integral between adjacent dopants. Since each dopant P atom contributes one valence electron, the impurity band is intrinsically 'half filled' (schematic in Fig. 1a), which reinforces the interaction effects due to the inbuilt electron-hole symmetry, and forms an ideal platform to explore the rich phenomenology of the 2D MottHubbard model, ranging from Mott metal-insulator transition (MIT) to novel spin excitations and magnetic ordering [14][15][16][17].In this Letter we show evidence of spontaneously broken time reversal symmetry in 2D Si:P and Ge:P δ-layers as the on-site effective Coulomb interaction is increased by decreasing the doping density of P atoms. Quantum transport and noise experiments indicate a strong suppression of quantum interference effects at low doping densities. We could attribute this to a spontaneous breaking of time reversal symmetry which manifest in an unambiguous suppression of universal conductance fluctuations (UCF) at zero magnetic fiel...