“…Nonlinear optical (NLO) devices, which function on the basis of photon–photon (p-p) interactions within nonabsorbing media, play a vital role in stimulating advanced applications in modern on-chip photonic integrated circuits (PICs). − Second harmonic generation (SHG), a typical nonlinear parametric process describing the frequency doubling of incident light, lies at the core of various nonlinear photonic hardware, such as optical switches, , optical modulators, , and optical quantum information processors. , Typically, for a material with a specific lattice structure, the excitation amplitude of SHG is proportional to the nonvanishing components in the second-order susceptibility tensor, which is strictly constrained by the point group symmetry that the material belongs to . Bulk crystals with noncentrosymmetric lattice structures, for example, β barium borate (β-Ba(BO 2 ) 2 ) and lithium niobate (LiNbO 3 ), have long been a central focus in developing SHG-related devices. , However, due to the inherently weak p-p interaction in these 3D classical media, achieving appreciable SHG response remains challenging within miniaturized interaction volumes under moderate light pumping, even though the strict phase-matching conditions are satisfied. , This inevitably hinders their integration in the state-of-the-art complementary metal-oxide-semiconductor (CMOS) compatible platform, which features continuous down-scaling with high power-efficiency. , …”