Growing population, increasing urbanization, and rural to urban migration, coupled with the ongoing climate change, threaten the sustainability of cities, particularly in developing countries. Previous studies indicate numerous deficiencies in the water supply and sewage systems of Islamabad; however, a comprehensive insight into the water security assessment has not been carried out. Therefore, this study is aimed at assessing the urban water security of Islamabad by taking both human and environmental aspects into consideration. In principle, we achieve this objective by implementing the Water Security Assessment Framework, using five distinct parameters to calculate an urban water security index. The water supply dimension incorporates availability, accessibility, affordability, and the quality of drinking water in the city, whereas, sanitation and health dimension measures access to improved drainage systems as well as the state of overall hygiene of the city inhabitants. Furthermore, the water economy dimension includes water productivity and investment aspects in the study area, while the environment and ecosystem dimension looks into the current state of natural water bodies. Similarly, overall management and public support for freshwater resources are measured in the society and governance dimension. In general, we attempt to better comprehend water-security nexus in the federal capital considering it as a prerequisite to ensure a sustainable future for the city dwellers.