Ornamental grasses are often used in gardens to improve biodiversity and as additional aesthetical resources. However, their use in green roofs (GR) and living walls (LW) is not so widespread and it has not been studied extensively. The aim of this work is to assess the performance of seven grass species (Imperata cylindrica ‘Red Baron’, Acorus gramineus, Stipa tenuissima ‘Pony Fails’, Carex flagellifera ‘Bronzita’, Carex oshimensis ‘Evergold’, Uncinia rubra ‘Everflame’ and Miscanthus sinensis) for their use in GR and LW. The growth of the plants was evaluated (i.e. biomass production, dimensions), as well as their visual quality and survival. C. flagellifera and C. oshimensis showed coverage levels greater than 75% and good visual quality, while A. gramineus reached 55–60%. I. cylindrica and M. sinensis showed coverages slightly below 50% in the LW, however, both performed well in the GR, though with a lower visual quality. U. rubra did not develop well, reaching the lowest coverage (below 45%) but maintaining a high visual quality. S. tenuissima also attained low coverage in the LW and presented high mortality, especially in the GR. In LW, C. oshimensis stood out in flowering, while S. tenuissima showed the highest flowering rate in GR. The species should be selected considering their characteristics and performance in order to achieve a correct appearance and development. Interspecific interactions are especially important in LW, as species with upward growth should be placed above species with fallen leaves, not below.