Interfacial engineering of lithium metal anodes: what is left to uncover?

Oyakhire, Solomon T.; Bent, Stacey F.

doi:10.1039/d3ya00470h

Energy Adv.

2024

DOI: 10.1039/d3ya00470h

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Interfacial engineering of lithium metal anodes: what is left to uncover?

Solomon T. Oyakhire,

Stacey F. Bent

Abstract: Lithium metal batteries possess remarkable energy storage capabilities, but their commercial realization is stifled by challenges in controlling the reactivity of lithium. Interfacial engineering has emerged as a promising approach...

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Cited by 2 publications

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Interfacial Engineering of Polymer Solid‐State Lithium Battery Electrolytes and Li‐Metal Anode: Current Status and Future Directions

Majeed,

Hussain,

Hussain

et al. 2024

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A combination of material innovations, advanced manufacturing, battery management systems, and regulatory standards is necessary to improve the energy density and safety of lithium (Li) batteries. High‐energy‐density solid‐state Li‐batteries have the potential to revolutionize industries and technologies, making them a research priority. The combination of improved safety and compatibility with high‐capacity electrode materials makes solid‐stateLi‐batteries with polymer solid‐electrolytes an attractive option for applications where energy density and safety are critical. While polymer‐based solid‐state Li‐batteries hold enormous promise, there are still several challenges that must be addressed, particularly regarding interface between polymer solid‐electrolyte and Lianode. There are significant advancements in improving the performance of solid‐state Li batteries, and researchers continue to explore new methods to address these challenges. These improvements are critical for enabling the widespread adoption of solid‐state Li‐batteries invariety of applications, from electrical vehicles to portable electronics. Here, common polymer solid‐electrolyte and its interface challenges with Lianode are first introduced, highlighting the trend in polymer solid‐state‐electrolyte research toward enhancing stability, safety, and performance of solid‐state Li‐batteries. This includes developing novel polymer materials with improved properties, exploring advanced fabrication techniques, and integrating these electrolytes into battery designs that optimize both safety and energy density.

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Interfacial Engineering of Polymer Solid‐State Lithium Battery Electrolytes and Li‐Metal Anode: Current Status and Future Directions

Majeed,

Hussain,

Hussain

et al. 2024

Small

View full text Add to dashboard Cite

show abstract

Double layer capacitance as a sensitive metric to monitor the formation of solid electrolyte interphases in Li–ion batteries

Schalenbach,

Wu,

Tsai

et al. 2025

Energy Adv.

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Interfacial engineering of lithium metal anodes: what is left to uncover?

Abstract: Lithium metal batteries possess remarkable energy storage capabilities, but their commercial realization is stifled by challenges in controlling the reactivity of lithium. Interfacial engineering has emerged as a promising approach...

Cited by 2 publications

References 109 publications

Interfacial Engineering of Polymer Solid‐State Lithium Battery Electrolytes and Li‐Metal Anode: Current Status and Future Directions

Interfacial Engineering of Polymer Solid‐State Lithium Battery Electrolytes and Li‐Metal Anode: Current Status and Future Directions

Double layer capacitance as a sensitive metric to monitor the formation of solid electrolyte interphases in Li–ion batteries

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