“…The excitation spectrum for generating 4-5 emission can be obtained by fixing the emission frequency ω = ω 45 and tuning the frequencies of the laser fields (I) and (II), respectively, near the 3S-3P and 3P-5S resonant transitions while the two-photon resonance condition be satisfied, that is, S( ) = Re (z, )| z=i ω 45 . In [16], the authors calculated the population in level 4 by perturbation expansion of the density matrix element ρ 44 up to the fourth order. In this paper, we do not calculate the population ρ 44 , but calculate the excitation spectrum for generating 5S-4P emission.…”