2009
DOI: 10.1103/physrevb.80.094524
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Interplay of rare earth and iron magnetism inRFeAsO(R=La, Ce, Pr, and Sm): Muon-spin relaxation study and symmetry analysis

Abstract: We report zero-field muon spin relaxation ͑SR͒ measurements on RFeAsO with R = La, Ce, Pr, and Sm. We study the interaction of the FeAs and R ͑rare-earth͒ electronic systems in the nonsuperconducting magnetically ordered parent compounds of RFeAsO 1−x F x superconductors via a detailed comparison of the local hyperfine fields at the muon site with available Mössbauer spectroscopy and neutron-scattering data. These studies provide microscopic evidence of long-range commensurate magnetic Fe order with the Fe mom… Show more

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Cited by 144 publications
(299 citation statements)
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References 51 publications
(128 reference statements)
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“…Both the FM and AF transitions are evident in the temperature derivative of the resistance but do not result in large anomalies as observed for RFeAsO. In the RFeAsO materials the Fe spins order in a striped pattern with a small ordered moment of ϳ0.4 B for all R from spectroscopic methods such as Mossbauer and SR. 25 Neutron powder diffraction, in contrast, suggests a wider spread of 0.3-0.8 B , 26 which Maeter et al have attributed to an induced magnetization on the R sublattice below T SDW that contributes to the "Fe" magnetic Bragg reflections. 25 It is not clear from our measurements whether this is important but the almost constant Co moment between 1.7 and 40 K ͑ ϳ0.3 B ͒ suggests that there is no significant induced "Nd contribution."…”
Section: Discussionmentioning
confidence: 99%
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“…Both the FM and AF transitions are evident in the temperature derivative of the resistance but do not result in large anomalies as observed for RFeAsO. In the RFeAsO materials the Fe spins order in a striped pattern with a small ordered moment of ϳ0.4 B for all R from spectroscopic methods such as Mossbauer and SR. 25 Neutron powder diffraction, in contrast, suggests a wider spread of 0.3-0.8 B , 26 which Maeter et al have attributed to an induced magnetization on the R sublattice below T SDW that contributes to the "Fe" magnetic Bragg reflections. 25 It is not clear from our measurements whether this is important but the almost constant Co moment between 1.7 and 40 K ͑ ϳ0.3 B ͒ suggests that there is no significant induced "Nd contribution."…”
Section: Discussionmentioning
confidence: 99%
“…In the RFeAsO materials the Fe spins order in a striped pattern with a small ordered moment of ϳ0.4 B for all R from spectroscopic methods such as Mossbauer and SR. 25 Neutron powder diffraction, in contrast, suggests a wider spread of 0.3-0.8 B , 26 which Maeter et al have attributed to an induced magnetization on the R sublattice below T SDW that contributes to the "Fe" magnetic Bragg reflections. 25 It is not clear from our measurements whether this is important but the almost constant Co moment between 1.7 and 40 K ͑ ϳ0.3 B ͒ suggests that there is no significant induced "Nd contribution." The spectroscopic measurements also suggest that the R spin ordering does not have any effect on the magnitude of the Fe moment, while for neutron powder diffraction increases have been reported, in particular, for R = Nd.…”
Section: Discussionmentioning
confidence: 99%
“…It was observed in the isostructural PrFeAsO where the in-plane stripe-like Fe AFM order is preserved but the Fe moments rotate to out-of-plane collinear AFM order below T Pr ≈ 11 K via Pr-Fe interaction. 11,14 Note that whereas the long-range Pr moments point along the c axis and the Fe moments rotate toward that axis in PrFeAsO, the long-range Ce moments are in the ab plane as discussed below and the Fe moments rotate in the ab plane in CeFeAsO, possibly reflecting the magnetic anisotropy of Fe sublattice by Ce magnetism via the Ce-Fe interaction in CeFeAsO. Based on our analysis, we cannot rule out the possibility that short-range Ce ordering slightly contributes to the anomaly at T * .…”
Section: Ce L Ii Rxms Measurementsmentioning
confidence: 99%
“…However, magnetization, resistivity and heat capacity measurements on polycrystalline 12 and single-crystalline 13 CeFeAsO have been interpreted in terms of very weak or no Ce-Fe exchange coupling. It is interesting to point out that as an outcome of the Pr-Fe coupling, the isostructural PrFeAsO exhibits temperature-induced Fe spin reorientation, 11,14 whereas for LaFeAsO involving nonmagnetic La, the Fe moments are fixed to be along the a axis even at low temperatures. 15 Moreover, temperature-induced Fe spin reorientation transition has been observed in few nonpnictide compounds involving rare-earth R and Fe sublattices, such as RFeO 3 , 16 RFe 2 , 16 RFe 11 Ti, 17 and R 2 Fe 14 B.…”
Section: Introductionmentioning
confidence: 99%
“…16,17 On the Co-rich side, the ferromagnetically ordered Co ions have a strong polarization effect on the AFM order of Ce moments. 14,18 On the other hand, in the Gd(Fe,Co)AsO series, which correspond to the case of a large 4f -magnetic moment, Fe/Co substitution also leads to a superconducting dome near the 3d-electron magnetic instability.…”
Section: Introductionmentioning
confidence: 99%