Disordered topological insulator (TI) films have gained
intense
interest by benefiting from both the TI’s exotic transport
properties and the advantage of mass production by sputtering. Here,
we report on the clear evidence of spin-charge conversion (SCC) in
amorphous Gd-alloyed Bi
x
Se1–x
(BSG)/CoFeB bilayers fabricated by sputtering, which
could be related to the amorphous TI surface states. Two methods have
been employed to study SCC in BSG (t
BSG = 6–16 nm)/CoFeB(5 nm) bilayers with different BSG thicknesses.
First, spin pumping is used to generate a spin current in CoFeB and
detect SCC by the inverse Edelstein effect (IEE). The maximum SCC
efficiency (SCE) is measured to be as large as 0.035 nm (IEE length λ
IEE) in a 6 nm thick BSG sample, which
shows a strong decay when t
BSG increases
due to the increase of BSG surface roughness. The second method is
THz time-domain spectroscopy, which reveals a small t
BSG dependence of SCE, validating the occurrence of a
pure interface state-related SCC. Furthermore, our angle-resolved
photoemission spectroscopy data show dispersive two-dimensional surface
states that cross the bulk gap until the Fermi level, strengthening
the possibility of SCC due to the amorphous TI states. Our studies
provide a new experimental direction toward the search for topological
systems in amorphous solids.