Two-dimensional
(2D) layered metal dichalcogenides constitute
a
promising class of materials for photodetector applications due to
their excellent optoelectronic properties. The most common photodetectors,
which work on the principle of photoconductive or photovoltaic effects,
however, require either the application of external voltage biases
or built-in electric fields, which makes it challenging to simultaneously
achieve high responsivities across broad-band wavelength excitationespecially
beyond the material’s nominal band gapwhile producing
low dark currents. In this work, we report the discovery of an intricate
phonon–photon–electron couplingwhich we term
the acoustophotoelectric effectin SnS2 that facilitates efficient photodetection through the application
of 100 MHz order propagating surface acoustic waves (SAWs). This effect
not only reduces the band gap of SnS2 but also provides
the requisite momentum for indirect band gap transition of the photoexcited
charge carriers, to enable broad-band photodetection beyond the visible
light range, while maintaining pA-order dark currents without
the need for any external voltage bias. More specifically, we show
in the infrared excitation range that it is possible to achieve up
to 8 orders of magnitude improvement in the material’s photoresponsivity
compared to that previously reported for SnS2-based photodetectors,
in addition to exhibiting superior performance compared to most other
2D materials reported to date for photodetection.