Recently, deep learning (DL) has emerged as a revolutionary and versatile tool transforming industry applications and generating new and improved capabilities for scientific discovery and model building. The adoption of DL in water science 20 has so far been gradual, but the related fields are now ripe for breakthroughs. This paper proposes that DL-based methods can open up a viable, complementary avenue toward knowledge discovery in hydrologic sciences. In the new avenue, machinelearning algorithms present competing hypotheses that are consistent with data for scientists to further evaluate. Interrogative studies are invoked to interpret DL models. In addition, we lay out several opinions shared by authors: (1) deep learning may bring forth transformative progress to the field of hydrology due to its ability to assimilate big data and identify commonalities 25 and differences; (2) the community may benefit greatly from a variety of shared datasets and open competitions; (3) big hydrologic data can be obtained via various ways including data compilation and working with citizen scientists, which offers the co-benefits of education and stakeholder engagement; (4) water sciences, and hydrology in particular, offer a unique set of challenges that can, in turn, stimulate advances in machine learning; and (5) An urgent need for research is hydrologycustomized methods for interpreting knowledge extracted by deep learning. 30Hydrol. Earth Syst. Sci. Discuss., https://doi.