nanomaterials with excellent electrical properties have been used in flexible piezoresistive force sensors, such as graphene, carbon nanotube (CNT), and graphite nanoplatelets. The electronic band structure of graphene is shifted by its in-plane elastic strain, which causes attractive changes in the electrical properties under structural deformation. [10] Uniform nanographene films obtained by chemical vapor deposition have been reported to exhibit a gauge factor of over 250, whereas the maximum strain was found to be less than 0.4%. [11,12] To achieve force sensors with a high stress sensitivity and a large strain range, macroscopic 3D monoliths of these nanomaterials with high porosity and compressibility have been developed. [13][14][15][16][17] Lv et al. demonstrated a simple sparkling strategy to produce ultralight graphene blocks. [15] Kim et al. transformed an inelastic CNT aerogel into a superelastic material by coating it with graphene nanoplatelets. [16,17] The above-mentioned 3D monoliths exhibit good electrical conductivity and high compressive strain ranges. However, the sparkling approach generates air bubbles with a size of 100-300 µm, forming a macroporous framework. The coating of CNT aerogel with graphene nanoplatelets involves the conversion of polyacrylonitrile into graphene at 1010 °C with the shrinkage of CNT aerogels. The fabrication of monoliths using the above-mentioned strategies has many challenges such as high temperatures and dimension shrinkage in microfabrication. These monoliths are all fabricated on the macroscale and face many challenges in microfabrication.Electrically conductive nanocomposites comprising carbonbased nanomaterials and insulating polymer matrices have been used in force sensors because of their excellent stretchability, low cost, and facile process of fabrication. [18][19][20][21] Owing to the universality of this technique and diverse mechanical properties of different polymers, the obtained conductive nanocomposites exhibit a wide range of elastic moduli. The dependence of electrical resistivity on force can be adjusted by changing the nanomaterial concentration. [22,23] To achieve a high sensitivity in the low-stress regime, porous structures and microdome/pyramid arrays have been developed. [24][25][26][27][28][29][30][31] Lee et al. fabricated an ultrasensitive pressure sensor by an electrospinning process, [30] and Park et al. demonstrated the detection of Flexible force sensors based on graphene/polymer nanocomposites have attracted tremendous attention owing to their remarkable sensitivity and ease of fabrication. In the present study, nanocomposites consisting of graphene as conducting fillers in a polyimide matrix are prepared, and an electrical breakdown method is used to endow the nanocomposite with a high piezoresistivity. Electromechanical tests and theoretical models confirm that the piezoresistivity of the nanocomposite originates from the cracks in the carbonized polymers induced by electrical breakdown. The fabricated force sensor exhibits a bro...