Abstract:The effects of water vapor and He
ion irradiation on the alteration
of particles of the uranyl hydroxide phase metaschoepite, [(UO2)8O2(OH)12](H2O)10, are determined. Raman spectra collected immediately
postirradiation revealed the presence of a uranyl oxide phase structurally
similar to γ-UO3 or U2O7. Short-term
storage postirradiation at elevated relative humidity accelerated
formation of the uranyl peroxide phase studtite, [(UO2)(O2)(H2O)2](H2O)2. Experiments examining the degradation of metaschoepite a… Show more
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