Investigation on Spectral Characteristics of Gliding Arc Plasma Assisted Ammonia Lean Combustion

Abstract

Ammonia as a non-carbon fuel is expected to play an important role in the future, but it is difficult to be effectively utilized at this stage due to its flame retardancy and other characteristics. Therefore, we propose to use gliding arc plasma combined with a swirl burner to enhance the combustion performance of ammonia. The electrical characteristics, electron density, gas rotational temperature and the distribution of key active species in the burner were studied via optical emission spectroscopy (OES). With the increase of equivalence ratio (EQR), the width of the Hα line decreases significantly, indicating that the electron density shows a downward trend, even as the gas rotational temperature shows an upward trend. When the equivalence ratio was 0.5, the gas rotational temperature increases by about 320 K compared with the pure air condition. During pure air discharge, there will still be obvious NO emission due to the plasma reaction, but with the addition of NH3, the NO content in the emission is significantly reduced. The light intensity of O atoms in the burner gradually decreases with the increase of the equivalence ratio, the light intensity of H atoms increases first and then decreases, and the light intensity of NH shows an upward trend. The reason may be that the plasma discharge effectively strengthens NH3(E)->NH2+H, NH2+H->NH+H2 and other reactions promote the initial reaction step of NH3 which thus effectively strengthens the NH3 combustion.

Experimental study on the discharge characteristics of an air rotating gliding arc

“…The gliding arc discharge is attracting increasing interest from worldwide researchers since it has been widely used in gas conversion and energy fields [1][2][3][4][5] due to the high energy efficiency, operating at atmospheric pressure and the simplicity of the discharge reactor. In recent years, many numerical simulations [6,7] and experiments [8][9][10] have been conducted to understand the gliding arc discharges for better sustainable applications.…”