Inorganic
transparent metal oxides represent one of the highest
performing material systems for thin-film flexible electronics. Integrating
these materials with low-temperature processing and printing technologies
could fuel the next generation of ubiquitous transparent devices.
In this work, we investigate the integration of UV-annealing with
inkjet printing, demonstrating how UV-annealing of high-k AlO
x
dielectrics facilitates the fabrication
of high-performance InO
x
transistors at
low processing temperatures and improves bias-stress stability of
devices with all-printed dielectrics, semiconductors, and source/drain
electrodes. First, the influence of UV-annealing on printed metal–insulator–metal
capacitors is explored, illustrating the effects of UV-annealing on
the electrical, chemical, and morphological properties of the printed
gate dielectrics. Utilizing these dielectrics, printed InO
x
transistors were fabricated which achieved exceptional
performance at low process temperatures (<250 °C), with linear
mobility μlin ≈ 12 ± 1.6 cm2/V s, subthreshold slope <150 mV/dec, I
on/I
off > 107, and minimal
hysteresis
(<50 mV). Importantly, detailed characterization of these UV-annealed
printed devices reveals enhanced operational stability, with reduced
threshold voltage (V
t) shifts and more
stable on-current. This work highlights a unique, synergistic interaction
between low-temperature-processed high-k dielectrics
and printed metal oxide semiconductors.