Ionic liquid gel microspheres as an emerging platform for constructing liquid compartment microreactors

He, Dongqing; Cao, Dezhou; Ben, Chuxuan; Lan, Yalin; Zhang, He; Jiang, Meijiao; Wu, Shuyao; Meng, Qing; Song, Xi‐Ming

doi:10.1039/d2gc01763f

Green Chem.

2022

DOI: 10.1039/d2gc01763f

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Ionic liquid gel microspheres as an emerging platform for constructing liquid compartment microreactors

Dongqing He

Dezhou Cao

Chuxuan Ben

et al.

Abstract: Flow chemistry technology innovatively integrates the traditional independent experimental operation processes, speeds up the reaction rate, specially, can carry out special reactions with danger or under difficult reaction conditions, being...

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2024

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Cited by 7 publications

References 74 publications

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Hydrophobic Ionic Liquid Gel Microspheres as Bi‐Component Carriers with a Liquid Phase to Immobilize Enzymes for Enhanced Performance

Ben,

Zhao,

et al. 2024

Adv Funct Materials

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This study focuses on incorporating liquid molecules, different from the bulk solution, into the immobilized enzyme carrier to regulate the distribution effect and diffusion‐limiting impact of the carrier's microenvironment for substrates, which generally is difficult to achieve due to the instability of the materials with liquid inclusions. A freestanding liquid‐holding particle carrier, with bi‐component hydrophobic ionic liquid gel microspheres with poly (glycidyl methacrylate) as the network and 1‐butyl‐3‐methylimidazolium hexafluorophosphate as the dispersing medium, is proposed, which is stable in air aqueous solution, and can extract proteins and organic small molecules into its interior due to the mobility of its dispersing medium. Horseradish peroxidase is covalently immobilized into the microspheres, forming a liquid compartment enzyme microreactor. The microreactor exhibits superior stability, enzymatic activity, and catalytic performance for Basic Orange II degradation compared to free enzyme and liquid‐free immobilized enzymes. This is attributed to the biocompatibility of the ionic liquid, its role in substrate enrichment in its interior, and its rapid mass transfer capability. This contribution shows the effectiveness of regulating the carrier's microenvironment with liquid molecules, offering fresh perspectives and strategies for enzyme technology.

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Hydrophobic Ionic Liquid Gel Microspheres as Bi‐Component Carriers with a Liquid Phase to Immobilize Enzymes for Enhanced Performance

Ben,

Zhao,

et al. 2024

Adv Funct Materials

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Acidic ionic liquid-based liposome for efficient catalytic degradation of azo dyes

Zhang,

Zheng

et al. 2024

Applied Surface Science

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Ionic liquid gel microspheres as multifunctional bi-component additives for the crystallinity manipulation and defect passivation in all-air-processed perovskite solar cells

Zeng,

Liu,

Wang

et al. 2024

Chemical Engineering Journal

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Ionic liquid gel microspheres as an emerging platform for constructing liquid compartment microreactors

Abstract: Flow chemistry technology innovatively integrates the traditional independent experimental operation processes, speeds up the reaction rate, specially, can carry out special reactions with danger or under difficult reaction conditions, being...

Cited by 7 publications

References 74 publications

Hydrophobic Ionic Liquid Gel Microspheres as Bi‐Component Carriers with a Liquid Phase to Immobilize Enzymes for Enhanced Performance

Hydrophobic Ionic Liquid Gel Microspheres as Bi‐Component Carriers with a Liquid Phase to Immobilize Enzymes for Enhanced Performance

Acidic ionic liquid-based liposome for efficient catalytic degradation of azo dyes

Ionic liquid gel microspheres as multifunctional bi-component additives for the crystallinity manipulation and defect passivation in all-air-processed perovskite solar cells

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