2022
DOI: 10.1016/j.jhazmat.2021.127763
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Iron single-atom anchored N-doped carbon as a ‘laccase-like’ nanozyme for the degradation and detection of phenolic pollutants and adrenaline

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Cited by 91 publications
(38 citation statements)
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“…This intermediate can undergo isomerization followed by subsequent dehydrogenation to give the complete dehydrogenated product 2a . Following previous suggestions, 28,54 the mechanism of this catalytic oxidative dehydrogenation may be similar to that of laccase oxidation of phenol, in which O 2 can be directly reduced to water by a four-electron transfer process.…”
Section: Resultsmentioning
confidence: 60%
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“…This intermediate can undergo isomerization followed by subsequent dehydrogenation to give the complete dehydrogenated product 2a . Following previous suggestions, 28,54 the mechanism of this catalytic oxidative dehydrogenation may be similar to that of laccase oxidation of phenol, in which O 2 can be directly reduced to water by a four-electron transfer process.…”
Section: Resultsmentioning
confidence: 60%
“…In fact, such materials have shown promising applications as catalysts in different organic reactions, [24][25][26] degradation of environmental pollutants, and electrochemical catalysis in the past decade. [27][28][29] To improve the catalytic activity of the pristine carbon materials, heteroatom doping (B, N, P, S, etc.) is a promising approach, which can effectively modulate the electronic structures, induce defects in lattices and produce active catalytic centers.…”
Section: Introductionmentioning
confidence: 99%
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“…[2] Most notably, among these phenolic components, bisphenol A (BPA) is banned from baby products in many countries, and 4-chlorophenol (4-CP) has been labeled as priority pollutants by the United States Environmental Protection Agency since 2009. [3,4] Multiple conventional strategies have been evolved to remove phenols from water, including adsorption and biodegradation. [5] Due to the stable structure and low biodegradability of target phenolic compounds, these methods are always challenged with the high cost, low efficiency, and generation of secondary contamination.…”
mentioning
confidence: 99%
“…To date, only a handful of examples using the ZIF-derived M@NCs as catalysts have been reported in several well-known organic transformations, including oxidation, 41 hydrogenation, 42 CO 2 fixation, 43 and further exploration of the applications of ZIF-derived M@NCs in developing more useful organic transformations appeared to be the best option owing to their simple synthetic procedure, tunable and uniform 3D porous structure, stable and dispersed metal sites, various metal–support interactions, excellent catalytic redox ability and so on. 44–46…”
Section: Introductionmentioning
confidence: 99%