“…2,3,5,6,18−22 Specifically, measurement of free electrons' energy can be used for the heralded generation of quantum light, such as Fock states, 1,4,8,10,23−25 squeezed states 26 and even cat and GKP states. 9 More recently, it was predicted that free electrons could serve as ancillary qubits for quantum computation 15,16 and provide a platform for nonlinear electron dynamics 27,28 and deterministic single-photon nonlinearities 11,29,30 emerging from quantum recoil. 31,32 Owing to the nature of free-electron emitters, the anticipated single photon nonlinearity can span a vast spectral range 33,34 and operate on femtosecond-temporal and subwavelength-spatial resolution, 35−37 allowing new paradigms in quantum optical technologies.…”