material, graphene has been widely employed in the fabrication of flexible strain sensors because of their outstanding electrical and mechanical properties and the as-prepared sensor has shown high sensitivity and great flexibility for diverse human motion monitoring. [7][8][9][10][11][12] Human motions monitoring can be divided into two categories: large human motions, such as bending/straightening of human joints, which can be used for analysis of motion patterns; and subtle human physiological motions, such as pulse, breath and speak, which can be used for human health assessment. [13][14][15][16] Large human joint motions usually result in about 55% strain, [7] and often require that the sensing material has a broad range of strain deformations and excellent stretchability to keep its structural connections at large strains. In contrast, subtle human motions usually induce about 1% strain, [7] demanding that the sensing material has high sensitivity. However, the strain sensors with high sensitivity easily lead to drastic structural changes at small deformation, and usually suffer a restricted strain range, whereas the strain sensors with high stretchability to detect large strain usually have poor sensitivity and cannot detect the subtle strains. To solve this issues, considerable effort has been devoted to developing strain sensors with high sensitivity and stretchability for detecting both large and subtle human motions. [13][14][15][16][17][18][19][20][21][22][23] Designing the geometric structures and controlling the connection types of graphene-sensing materials are the main approaches to realizing these goals. For example, Ren et al. recently proposed on using a laser-patterned graphene-sensing film for fabrication of a high performance strain sensor, where sensitivity and strain range can be adjusted by the patterns of the graphene for detecting both large and subtle human motions. [13] Shi et al developed a fish scale-like graphene-sensing layer for highly sensitive and large-range strain sensors, and they exhibited a wide sensing range (up to 82% strain) and high sensitivity with a gauge factor (GF) of 16.2 within 60% strain for full-range human motions detection. [14] Furthermore, two-order open mesh graphene film, [15] graphene armor scales [16] and silver nanoparticles bridge graphene film [17] have been also employed for highly sensitive and large-range strain sensors for both large and subtle human Wearable strain sensors with high sensitivity and broad sensing ranges to detect both subtle and large human motion are highly desirable in health monitoring systems. Here, a novel, dual-mode strain sensor based on the reduced graphene oxide (rGO)/polydimethlsiloxane (PDMS) film adhered to micropatterning elastomer colloidal crystal film is proposed to realize these goals. The rGO/PDMS film is designed for detecting subtle human motion via its resistance change, while the colloidal crystal film is used for detecting large human motion via its simple colorimetric changes or reflection peak shifts and ...