2000
DOI: 10.1103/physrevlett.84.1990
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Large Isotope Effect on the Pseudogap in the High-Temperature SuperconductorHoBa2Cu4O8

Abstract: The oxygen isotope effect on the relaxation rate of crystal-field excitations in the slightly underdoped high-temperature superconductor HoBa2Cu4O8 has been investigated by means of inelastic neutron scattering. For the 16O compound there is clear evidence for the opening of an electronic gap in the normal state at T(*) approximately 170 K far above T(c) = 79 K. Upon oxygen isotope substitution ( 16O vs 18O) T(c) decreases marginally to 78.5 K, whereas T(*) is shifted to about 220 K. This huge isotope shift ob… Show more

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Cited by 190 publications
(140 citation statements)
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“…This mean-field scheme treats the local dynamical atomic displacements as correlated to the local density fluctuations between the electrons and the bipolarons, which in our model, are responsible for the opening of the pseudogap. It is this mecha-nism which is at the origin of the blockage of the crystal field excitations which below T * couple to the free charge carriers, as observed experimentally in neutron spectroscopic measurements testing the transitions between different crystal field levels 8,9 . A more quantitative analysis than the mean-field procedure presented here would be required in order to account for the dynamical nature of the onset of pairing, as seen in experiments with different time scales 17 which lead to different absolute values of T * but to qualitatively similar doping dependence of T * .…”
Section: Discussionmentioning
confidence: 99%
“…This mean-field scheme treats the local dynamical atomic displacements as correlated to the local density fluctuations between the electrons and the bipolarons, which in our model, are responsible for the opening of the pseudogap. It is this mecha-nism which is at the origin of the blockage of the crystal field excitations which below T * couple to the free charge carriers, as observed experimentally in neutron spectroscopic measurements testing the transitions between different crystal field levels 8,9 . A more quantitative analysis than the mean-field procedure presented here would be required in order to account for the dynamical nature of the onset of pairing, as seen in experiments with different time scales 17 which lead to different absolute values of T * but to qualitatively similar doping dependence of T * .…”
Section: Discussionmentioning
confidence: 99%
“…Similarly, a large copper-isotope effect on T p has been found in the same compound [53]. The huge oxygen-isotope effects on T * [50] and on T p [52] indicate that a strong electron-phonon interaction plays an essential role in the charge dynamics and superconductivity [48]. Although the authors of Ref.…”
Section: Huge Oxygen-isotope Effect On the Charge Stripe Formationmentioning
confidence: 98%
“…From the figure, one can clearly see that, upon replacing 16 O with 18 O, the chargestripe formation temperature T * in this cuprate increases from about 110 K to 180 K. Such a large negative isotope effect on charge ordering can be explained in terms of electron-phonon coupling beyond the Migdal approximation [51]. Recently, a neutron spectroscopic investigation of the isotope effect on the relaxation rate of crystal field excitations of Ho 3+ in HoBa 2 Cu 4 O 8 has been carried out [52]. In Fig.…”
Section: Huge Oxygen-isotope Effect On the Charge Stripe Formationmentioning
confidence: 99%
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“…An even greater puzzle than the isotope effect on T c is the recently discovered one on T* [20][21][22]. Here the isotope effect is giant -one of the largest ever observed in solid state systems -and has most interestingly the reversed sign, i.e.…”
Section: Figure 51 the Doping Dependent Phase Diagram Of Htscmentioning
confidence: 99%