The ability of the rotary slingers to achieve fuel atomization by employing the rotational speed of the turbine shaft obviates the use of high-pressure fuel pump and makes those a popular choice for small gas turbine engines. Such atomizers contain arrays of orifices on their outer periphery for injection of the liquid into the combustion chambers. In the present work, we experimentally investigate the influence of the choice of orifice size on primary liquid breakup dynamics and spray characteristics in slinger atomizers. Three slinger discs with the same disc size and number of orifices but with different orifice size, d o (= 1 mm, 1.5 mm, and 2 mm) are examined in a high-speed slinger test rig for a range of rotational speed (2000–10,000 rpm) and liquid feed rate (0.2–1 lpm). The operating conditions are relevant to part-load and engine relighting conditions for which the selection of geometric parameters of the injector may play a crucial role in achieving the atomizer performance. In the current work, the liquid breakup process in the vicinity of the slinger orifices was visualized using front light illumination technique, whereas the pulse-shadowgraph technique was employed for droplet sizing. It is found that smaller orifice size promotes column mode of liquid breakup which results in larger primary liquid breakup length and subsequently results in larger Sauter mean diameter. The results highlight that the orifice size is an important design parameter as the liquid atomization in slinger atomizers is sensitive to the selection of orifice size especially for lower range of rotational speeds.