“…Particles which contribute most significantly to natural light scattering in the atmosphere are those of about V2 µ in diam (Pueschel and Noll, 1967), and for aerosols of approximately this size the scattering is nearly proportional to the particle volume (Charlson et al, 1967;Cooper and Byers, 1970). The volume mean diameters of the aerosols used in this work were approximately 0.2-0.4 µ and the volume median diameters were 0.6-1.5 µ. Measurements made by Whitby et al (1972) in Pasadena, Calif., gave a bimodal size distribution for the atmospheric aerosol, which in the light-scattering size region approximated a log-normal distribution of 0.3-µ median diam and 2.25 geometric std dev, quite similar to the aerosols used here.…”