Lattice Charge Tuning-Driven Multi-Carbon Products from Carbon Dioxide

Chawla, Geetansh; Sarma, Saurav Ch.; Raj, Jithu; Bagchi, Debabrata; Riyaz, Mohd; Roy, Soumyabrata; Mishra, Vidyanshu; Goud, Devender; Peter, Sebastian C.

doi:10.1021/acssuschemeng.4c02069

ACS Sustainable Chem. Eng.

2024

DOI: 10.1021/acssuschemeng.4c02069

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Lattice Charge Tuning-Driven Multi-Carbon Products from Carbon Dioxide

Geetansh Chawla,

Saurav Ch. Sarma,

Jithu Raj

et al.

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A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals

Mondal,

Peter

2024

Advanced Materials

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Electrochemical CO2 reduction reaction (eCO2RR) has been explored extensively for mitigation of noxious CO2 gas generating C1 and C2+ hydrocarbons and oxygenates as value‐added fuels and chemicals with remarkable selectivity. The source of CO2 being a pure CO2 feed, it does not fully satisfy the real‐time digestion of industrial exhausts. Besides the detrimental effect of noxious gas mixture leading to global warming, there is a huge capital investment in purifying the flue gas mixtures from industries. The presence of other impurity gases affects the eCO2RR mechanism and its activity and selectivity toward C2+ products dwindle drastically. Impurities like NOx, SOx, O2, N2, and halide ions present in flue gas mixture reduce the conversion and selectivity of eCO2RR significantly. Instead of wiping out these impurities via separation processes, new strategies from material chemistry and electrochemistry can open new avenues for turning foes to friends! In this perspective, the co‐electroreduction will vividly discussed and supporting role of different heteroatom‐containing impurity gases with CO2, generating highly stable C─N, C─S, C─X bonds, and highlight the existing limitations and providing probable solutions for attaining further success in this field and translating this to industrial exhaust streams.

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A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals

Mondal,

Peter

2024

Advanced Materials

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Lattice Charge Tuning-Driven Multi-Carbon Products from Carbon Dioxide

Cited by 1 publication

References 50 publications

A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals

A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals

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Lattice Charge Tuning-Driven Multi-Carbon Products from Carbon Dioxide

Cited by 1 publication

References 50 publications

A Perspective on Electrochemical Point Source Utilization of CO2 and Other Flue Gas Components to Value Added Chemicals

A Perspective on Electrochemical Point Source Utilization of CO2 and Other Flue Gas Components to Value Added Chemicals

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A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals

A Perspective on Electrochemical Point Source Utilization of CO₂ and Other Flue Gas Components to Value Added Chemicals