1993
DOI: 10.1007/bf01426757
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Lifetime measurements of highly excited Rydberg states of strontium I

Abstract: Abstract. Lifetimes of Rydberg states of the triplet-series 5s ns 3S 1 with n= 19-23, 35 and 5s nd 3D 3 with n= 18-20, 23-28 in the spectrum of neutral strontium have been determined. Observation of the exponential decay after excitation by a pulsed laser in a fast atomic beam and subsequent state-selective field ionization was employed. The lifetimes of the states of the 3Sl-series show the expected n* 3 dependence on the effective principal quantum number, while the 3D3-series is disturbed by configuration m… Show more

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Cited by 17 publications
(16 citation statements)
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“…5 again revealed near exponential decay. For the 38 3 S 1 atoms γ ′ TOT = 3.1×10 4 s −1 yielding the BBR-induced decay rate, γ BBR ≈ γ TOT − γ ′ TOT , ∼1.7×10 4 s −1 , a value in good agreement with that calculated using the TAE model, γ BBR = 1.4×10 4 s −1 , and one that is consistent with those reported previously in earlier studies of interactions between BBR and Rydberg atoms [17][18][19]. The effective lifetime of 20 µs calculated using the TAE model is also in good agreement with the measured value of 21(1) µs, although both values are substantially larger than the value reported previously for the 35 3 S 1 state of 7.5(44) µs [20].…”
Section: Resultssupporting
confidence: 90%
“…5 again revealed near exponential decay. For the 38 3 S 1 atoms γ ′ TOT = 3.1×10 4 s −1 yielding the BBR-induced decay rate, γ BBR ≈ γ TOT − γ ′ TOT , ∼1.7×10 4 s −1 , a value in good agreement with that calculated using the TAE model, γ BBR = 1.4×10 4 s −1 , and one that is consistent with those reported previously in earlier studies of interactions between BBR and Rydberg atoms [17][18][19]. The effective lifetime of 20 µs calculated using the TAE model is also in good agreement with the measured value of 21(1) µs, although both values are substantially larger than the value reported previously for the 35 3 S 1 state of 7.5(44) µs [20].…”
Section: Resultssupporting
confidence: 90%
“…However, the decay rate of the excited state is less well known. We obtain the best agreement with our data using a decay rate of (Γ 21 + Γ 2Loss ) = 310 × 10 3 s −1 , which is slightly higher than the natural decay rate expected from scaling the results of [59]. The branching ratio calculated from the Wigner-Eckart theorem would imply that 1/3 of the decays from the Rydberg state result in 3 P 1 atoms, but the recoil energy for a single 320 nm photon exceeds the trap depth, so we assume all radiative decay leads to atom loss and set Γ 21 = 0.…”
Section: Experimental Methodssupporting
confidence: 79%
“…We excite atoms exclusively to the 5s24s 3 S 1 Rydberg state (lifetime τ3 S1 ≈ 4µs [59]) with two-photon excitation using the narrow 1 S 0 → 3 P 1 transition (τ3 P1 = 21 µs) as the intermediate state ( Fig. 1).…”
Section: Experimental Methodsmentioning
confidence: 99%
“…. 100 have sizable lifetimes on the order of τ r ∼ 10 2 µs [46], which is a crucial feature of Rydberg atoms for their application in quantum information processing [47]. In the present situation, however, the production of large-N squeezed states requires even longer coherence times.…”
Section: Pacs Numbersmentioning
confidence: 99%