2009
DOI: 10.1103/physrevlett.102.015502
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Lifetime of THz Acoustic Nanocavity Modes

Abstract: We present an ultrahigh resolution Raman study of the lifetime of 1 THz acoustic phonons confined in nanocavities. We demonstrate that the cavity Q factor can be controlled by design. Anharmonicity contributes only marginally to limit the cavity phonon lifetime, even at room temperature, while thickness fluctuations in the scale of 1/10 of a unit cell are the main limitation for the performance of THz phonon cavities.

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Cited by 71 publications
(74 citation statements)
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“…It should be noted that unlike spectroscopic techniques [11][12][13][14][15] capable of measuring the lifetime of a specific phonon state within the Brillouin zone, our measurements do not provide such direct MFP information. Rather, we obtain integrated information on phonon MFPs and dispersion according to Eq.…”
mentioning
confidence: 89%
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“…It should be noted that unlike spectroscopic techniques [11][12][13][14][15] capable of measuring the lifetime of a specific phonon state within the Brillouin zone, our measurements do not provide such direct MFP information. Rather, we obtain integrated information on phonon MFPs and dispersion according to Eq.…”
mentioning
confidence: 89%
“…Although the frequency-dependence of phonon lifetimes can be measured directly with inelastic neutron [11], x-ray [12], or light scattering [13], or with laser-excited coherent phonons [14,15], MFP measurements by these techniques have been limited. For example, the available experimental data for silicon do not extend beyond 100 GHz [16], far below the range of frequencies thought to be important for thermal transport at room temperature [8,10] In recent years, advances in measuring phonon MFP distributions have been made with studies of size-dependent thermal conductivity over small distances, where thermal transport deviates from Fourier's law.…”
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confidence: 99%
“…Both types of modes are simultaneously observed in microcavities due to the standing wave character of the confined electromagnetic field. 40,42 As evidenced from these data, the larger intensity of the Raman peaks concentrates close to the branch's anticrossing, that is, when polaritons display similar excitonic and photonic character.…”
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confidence: 69%
“…To simplify the Raman experiments the frequency of the mechanical vibrations has been pushed up from the 20 GHz of the basic optomechanical mode of the microcavity as a whole, 22 to 250 GHz by replacing the bulk GaAs spacer of the optical microcavity by an acoustic multilayer. 39,42 The latter mostly consists of a 32 period GaAs/AlAs (14.16/5.81 nm) multiple quantum well (MQW). The experiments reported here have been performed in strong resonance with the GaAs exciton of these MQW at 1.53 eV.…”
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confidence: 99%
“…These conditions are far from reach with current devices, and to enhance the nonlinearity several alternative techniques have been proposed [18][19][20]. These approaches still require large optomechanical coupling rates GaAs/AlAs superlattice cavities, where a λ/2 cavity is enclosed by two distributed Bragg reflector (DBR) mirrors, can simultaneously confine the light field and the mechanical field [21,22]. The great advantage of superlattice planar cavities is that the large overlap between both optical and vibrational fields in the cavity region and the photoelastic effect leads to high optomechanical coupling rates [21].…”
Section: Introductionmentioning
confidence: 99%