“…In recent years, various self-oscillating systems based on diverse stimuli-responsive materials are reported, such as hydrogels [ 14 , 15 ], dielectric elastomers [ 16 ], ionic gels [ 17 ], liquid crystal elastomers (LCEs) [ 7 , 18 , 19 , 20 , 21 ], and thermally responsive polymer materials [ 22 ], etc. Furthermore, a variety of self-sustained motion modes have been constructed, such as bending [ 23 , 24 , 25 , 26 ], buckling [ 27 , 28 , 29 , 30 ], torsion [ 31 , 32 ], stretching and shrinking [ 33 , 34 ], rolling [ 35 , 36 ], swimming [ 9 ], swinging [ 37 , 38 ], vibration [ 39 , 40 , 41 ], jumping [ 42 , 43 , 44 ], rotation [ 45 ], eversion or inversion [ 46 , 47 ], and even synchronized motion of several coupled self-oscillators [ 48 ]. These self-sustained motions often originate from nonlinear feedback mechanisms including self-shadowing [ 3 , 27 , 28 ], coupling of liquid volatilization and membrane deformation [ 49 ], coupling mechanism among air expansion and liquid column movement [ 50 ], and coupling of plate buckling and chemical reaction [ 18 ].…”