Abstract. In this work, solar¯are energetic particlē uxes (E e ³ 42 keV) observed by the HI-SCALE instrument onboard Ulysses, a spacecraft that is probing the heliosphere in 3-D, are utilized as diagnostics of the large-scale structure and topology of the interplanetary magnetic ®eld (IMF) embedded within two well-identi®ed interplanetary coronal mass ejection (ICME) structures. On the basis of the energetic solar¯are particle observations ®rm conclusions are drawn on whether the detected ICMEs have been detached from the solar corona or are still magnetically anchored to it when they arrive at 2.5 AU. From the development of the angular distributions of the particle intensities, we have inferred that portions of the ICMEs studied consisted of both open and closed magnetic ®eld lines. Both ICMEs present a ®lamentary structure comprising magnetic ®laments with distinct electron anisotropy characteristics. Subsequently, we studied the evolution of the anisotropies of the energetic electrons along the magnetic ®eld loop-like structure of one ICME and computed the characteristic decay time of the anisotropy which is a measure of the amount of scattering that the trapped electron population underwent after injection at the Sun.