“…Calculations were performed with beginning-of-cycle (BOC) and end-of-cycle (EOC) conditions to bound typical HFIR operating conditions. The EOC inputs were obtained from previous depletion studies [1] performed with VESTA [10], a Monte Carlo-based depletion tool developed and maintained at Institut de Radioprotection et de Sûreté Nucléaire (French Institute for Radiological Protection and Nuclear Safety), which was validated against HFIR post-irradiation, spatially dependent uranium isotopic measurements [11] and compared to calculations performed with the Standardized Computer Analysis for Licensing Evaluations code package (SCALE) [12] in [13]. The fuel, CEs, and curium targets (applicable only to the LEU inputs) were depleted, and CE withdrawal was simulated during the VESTA calculations.…”