Abstract. To constrain uncertainties in radiative forcings associated with
aerosol–cloud interactions, improved understanding of Arctic cloud formation
is required, yet long-term measurements of the relevant cloud and aerosol
properties remain sparse. We present the first long-term study of cloud
residuals, i.e. particles that were involved in cloud formation and cloud
processes, in Arctic low-level clouds measured at Zeppelin Observatory,
Svalbard. To continuously sample cloud droplets and ice crystals and separate
them from non-activated aerosol, a ground-based counter-flow virtual impactor
inlet system (GCVI) was used. A detailed evaluation of the GCVI measurements,
using concurrent cloud particle size distributions, meteorological parameters,
and aerosol measurements, is presented for both warm and cold clouds, and the
potential contribution of sampling artefacts is discussed in detail. We find
an excellent agreement of the GCVI sampling efficiency of liquid clouds using
two independent approaches. The 2-year data set of cloud residual size
distributions and number concentrations reveals that the cloud residuals
follow the typical seasonal cycle of Arctic aerosol, with a maximum
concentration in spring and summer and a minimum concentration in the late
autumn and winter months. We observed average activation diameters in the
range of 58–78 nm for updraught velocities below 1 m s−1. A
cluster analysis also revealed cloud residual size distributions that were
dominated by Aitken mode particles down to around 20–30 nm. During
the winter months, some of these small particles may be the result of ice,
snow, or ice crystal shattering artefacts in the GCVI inlet; however, cloud
residuals down to 20 nm in size were also observed during conditions
when artefacts are less likely.