We have investigated the magnetization reversal behavior in exchange-coupled NiO/Fe films with varying the NiO thicknesses using a magneto-optical microscope magnetometer capable of direct domain observation in real time. Interestingly enough, the magnetization reversal mechanism is gradually changed from a domain wall-motion process to a nucleation process as the NiO thickness increases. This result clearly demonstrates that the exchange coupling effect between the NiO and Fe layers increases the domain wall pinning effect of the Fe layer, resulting in the nucleation reversal mode.The antiferromagnetic ͑AFM͒/ferromagnetic ͑FM͒ bilayer exhibits the coercive field enhancement and the loop shift in the magnetic hysteresis loop of the FM layer, known as the exchange coupling effect. 1 The exchange-coupled system has been largely studied due to their technical application as the pinned layer in a magnetoresistive spin-valve structure. 2-4 However, despite its extensive technical application, the physics of exchange coupling effect is not clearly understood yet. [5][6][7][8][9] Recently, several studies have focused on the change in magnetization reversal mechanism in a FM layer. [10][11][12][13] In general, the change in magnetization reversal mechanism could be explained by the increased domain wall ͑DW͒ pinning effect in a FM layer. 14-16 Since the DW pinning effect can be greatly affected by the t AFM , 17 it is necessary to measure magnetization reversal behavior with varying the AFM thicknesses ͑t AFM ͒ systematically to elucidate the origin of reversal mechanism change. The reliable study focusing on the correlation between reversal mechanism and t AFM was already carried out in NiO/Co system 18,19 through dynamical magnetization measurements from the hysteresis loop measured by means of the magneto-optical Kerr effect ͑MOKE͒ experimental setup. However, the MOKE method used in this experiment cannot reveal the detailed domain configuration during magnetization reversal. Since the domain reversal patterns can give the detailed information on the DW pinning effect, it is crucial to investigate the magnetization reversal behavior using the direct domain observation technique to extend our understanding on this issue.In this work, we have investigated the magnetization reversal behavior in exchange-coupled NiO/Fe films with varying NiO thicknesses using a magneto-optical microscope magnetometer ͑MOMM͒ capable of direct domain observation. 20 From the time-resolved domain images obtained by the MOMM, we have compared the magnetization reversal mechanism at each sample. Interestingly, the magnetization reversal mechanism in the NiO/Fe systems becomes changed from a wall-motion dominant process to a nucleation dominant one as the NiO thickness increases.For this study, we have prepared a series of the t NiO nm NiO/30 nm Fe samples with different thicknesses of t NiO =0, 30, 100, and 200 nm using a magnetron sputtering method under a base pressure of 2 ϫ 10 −6 Torr and an Ar sputtering pressure of 5 mTorr. The NiO and...