2021
DOI: 10.1002/aic.17263
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Mass transfer in 3D‐printed electrolyzers: The importance of inlet effects

Abstract: This article investigates the effect of inlet shape, entrance length, and turbulence promoters on mass transfer by using 3D-printed electrolyzers. Our results show that the inlet design can promote turbulence and lead to an earlier transition to turbulent flow. The Reynolds number at which the transition occurs can be predicted by the ratio of the cross-sectional area of the inlet to the cross-sectional area of the electrolyzer channel. A longer entrance length results in more laminar behavior and a later tran… Show more

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Cited by 12 publications
(3 citation statements)
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“…Previous work has highlighted the outsized effect that inlet and outlet design have on small scale electrochemical cells, as the flow is often not fully developed within the full active area. 35,36 These issues are exacerbated in a two-phase flow system where bubbles can complicate fluid interactions with manifolds or turbulence promoters. When comparing the cells with the pentagonal spacer and rectangular spacer, the CO 2 evolved on the anode side was nearly identical (see Fig.…”
Section: Resultsmentioning
confidence: 99%
“…Previous work has highlighted the outsized effect that inlet and outlet design have on small scale electrochemical cells, as the flow is often not fully developed within the full active area. 35,36 These issues are exacerbated in a two-phase flow system where bubbles can complicate fluid interactions with manifolds or turbulence promoters. When comparing the cells with the pentagonal spacer and rectangular spacer, the CO 2 evolved on the anode side was nearly identical (see Fig.…”
Section: Resultsmentioning
confidence: 99%
“…20 3D printing has been developed as a promising manufacturing technology in chemical research, 21 and particularly, in electrochemistry. 22,23 A wide range of cell components can be 3D printed: flow channels and turbulence promoters, 24,25 textured planar electrodes, 20,26,27 mesh-like electrodes, 28,29 and other porous electrodes. 30,31 3D printing is a helpful fast prototyping tool, reducing the costs and lead time associated in making individual pieces, while keeping adequate manufacture tolerances.…”
Section: Introductionmentioning
confidence: 99%
“…Nevertheless, recent progress in electrochemical process applications demands the use of different reactor designs and configurations for specific electrochemical processes. In electrochemical reactors composed of flat electrodes, the implementation of new flow distributor configurations is a required task to improve the performance of this kind of reactor, particularly by enhancing the mass transport uniformity over the electrode surface, 7 minimizing the costs, and pressure drop, among other aspects.…”
Section: Introductionmentioning
confidence: 99%