Material balances of carbon, sulfur, nitrogen and ilmenite in a 100kW CLC reactor system

Linderholm, Carl Johan; Knutsson, Pavleta; Schmitz, Matthias; Markström, Pontus; Lyngfelt, Anders

doi:10.1016/j.ijggc.2014.05.001

Cited by 67 publications

(47 citation statements)

References 31 publications

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“…A pilot operation using ilmenite suggested a life of 600-700 h [21] based on the production of fines. This lifetime estimation does not consider any interaction with ash, and a more realistic lifetime is probably 100-300 h. With ilmenite and assuming a lifetime of 200 h, the cost is 2 €/tonne CO 2 , Table 11.…”

Section: Oxygen Carrier Costmentioning

confidence: 99%

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A 1000 MWth boiler for chemical-looping combustion of solid fuels – Discussion of design and costs

2015

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h i g h l i g h t sChemical-Looping Combustion (CLC) is a novel combustion technology for CO 2 capture. CLC avoids large costs and energy penalties of gas separation for CO 2 capture. A scale-up of CLC technology for solid fuels to 1000 MW th is investigated. CLC technology is similar to CFB technology. Estimated cost of CLC with capture relative to CFB without capture is 20 €/tonne CO 2 . a b s t r a c tMore than 2000 h of solid-fuel CLC operation in a number of smaller pilot units clearly indicate that the concept works. A scale-up of the technology to 1000 MW th is investigated in terms of mass and heat balances, flows, solids inventories, boiler dimensions and the major differences between a full-scale Circulating Fluidized-Bed (CFB) boiler and a Chemical-Looping Combustion CFB (CLC-CFB). Furthermore, the additional cost of CLC-CFB relative to CFB technology is analysed and found to be 20 €/tonne CO 2 . The largest cost is made up of compression of CO 2 , which is common to all capture technologies. Although the need for oxygen to manage incomplete conversion is estimated to be only a tenth of that of oxy-fuel combustion, oxygen production is nonetheless the second largest cost. Other significant costs include oxygen-carrier material, increased boiler cost and steam for fluidization of the fuel reactor.

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Section: Oxygen Carrier Costmentioning

confidence: 99%

“…The first operation using solid fuels in a 10 kW unit was realized in 2006 [11] and today, a number of published articles address CLC pilot operation using solid fuel, e.g. [12][13][14][15][16][17][18][19][20][21].…”

Section: Introductionmentioning

confidence: 99%

A 1000 MWth boiler for chemical-looping combustion of solid fuels – Discussion of design and costs

2015

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“…Among the tested materials, ilmenite, iron-titanium mineral has been most widely tested within the performed CLC research [12,[16][17][18][19][20][21][22].…”

Section: Introductionmentioning

confidence: 99%

Characterization of ilmenite used as oxygen carrier in a 100 kW chemical-looping combustor for solid fuels

Knutsson

Linderholm

2015

Applied Energy

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“…However, large scale commercial CFB technology has been difficult to develop. Among the technical challenges related to CFB are the reactor cooling, looping seal design, and high steady recycle sorbent or oxygen carriers particles, etc (Linderholm et al, 2014;Ma et al, 2015;Romano et al, 2013).…”

Section: Economic Feasibilitymentioning

confidence: 99%

Comparison of carbon capture IGCC with chemical-looping combustion and with calcium-looping process driven by coal for power generation

Zhu

Jiang

Fan

2015

Chemical Engineering Research and Design

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Material balances of carbon, sulfur, nitrogen and ilmenite in a 100kW CLC reactor system

Cited by 67 publications

References 31 publications

A 1000 MWth boiler for chemical-looping combustion of solid fuels – Discussion of design and costs

A 1000 MWth boiler for chemical-looping combustion of solid fuels – Discussion of design and costs

Characterization of ilmenite used as oxygen carrier in a 100 kW chemical-looping combustor for solid fuels

Comparison of carbon capture IGCC with chemical-looping combustion and with calcium-looping process driven by coal for power generation

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