“…Recently, the thick film ceramic preparation processes, such as, screen printing, tape casting have been used to prepare PZT and related materials. [1][2][3][4][5] Tape casting is a convenient and useful method for the large-scale preparation of ceramic substrates, capacitors, and multilayered structural composites for various applications, such as: Al 2 O 3 , 6,7 AlN 8,9 substrates, BaTiO 3 capacitors, 10,11 solid electrolytes, [12][13][14] solid oxide fuel cells, [15][16][17][18][19][20] or PZT and PZST ceramic sheets. [21][22][23][24][25] In the past, the traditional tape casting focused on organic solvent systems due to their low latent heat of evaporation and low surface tension.…”