Noise measurements in light water reactor systems aid in generating validation data for integral point kinetic parameter predictions and generating monitoring parameters for reactor safety and safeguards. The CROCUS zero-power reactor has been used to support both efforts via measurements with thermal neutron detectors to observe neutron noise and inorganic scintillators to observe gamma noise. The cross-correlation of gamma and neutron noise has been investigated at CROCUS with separate gamma-only and neutron-only detectors. Organic scintillators, sensitive to both neutrons and gamma rays, can be used to cross-correlate gamma-ray and neutron noise with a single detector type. Herein, we present noise measurements using organic scintillators in a light-water, zero-power research reactor for the first time. We discuss data obtained with two 5.08 cm-length by 5.08 cm-diameter cylindrical trans-stilbene detectors and two 6-mm cubic scintillators -one trans-stilbene and one organic glass -set in the water reflector of CROCUS and outside the reactor vessel. The prompt neutron decay constant was estimated to be α CPSD = (154 ± 1) s −1 at 3 mW critical from the (γ,γ) signal, which agrees within one standard deviation overlap with previous measurements with CeBr3 and simulation in Serpent 2. The (n,n) estimate of α CPSD = (145 ± 23) s −1 at 3 mW critical lacked precision but agreed within one standard deviation overlap with previous 235 U fission chamber estimates and simulation in Serpent 2. The 6-mm cubic scintillators were too inefficient to estimate α, but informed possible small-cell, high-volume detection systems to improve the (n,n) estimate capabilities. Based on the high precision estimate of α from the (γ,γ) CPSD signal we suggest the further development of theory to calculate β eff and Λ from gamma-ray noise measurements and recommend gamma noise measurements for future simulation validation and as a method of reactor monitoring.