Measuring Mass Transfer of <i>n</i>-Hexane and 2-Chloroethyl Ethyl Sulfide in Sorbent/Polymer Fiber Composites Using a Volumetric Adsorption Apparatus

Son, Florencia A.; Shi, Kaihang; Snurr, Randall Q.; Farha, Omar K.

doi:10.1021/acsami.4c02117

ACS Appl. Mater. Interfaces

2024

DOI: 10.1021/acsami.4c02117

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Measuring Mass Transfer of n-Hexane and 2-Chloroethyl Ethyl Sulfide in Sorbent/Polymer Fiber Composites Using a Volumetric Adsorption Apparatus

Florencia A. Son,

Kaihang Shi,

Randall Q. Snurr

et al.

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2024

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Kinetics of Adsorption-Induced Deformation of Microporous Carbons

Kolesnikov,

Shkolin,

Men’shchikov

et al. 2024

Langmuir

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Equilibrium and kinetic behavior of adsorption-induced deformation have attracted a lot of attention in the last few decades. The theoretical and experimental works cover activated carbons, coals, zeolites, glasses, etc. However, most of the theoretical works describe only the equilibrium part of the deformation process or focus on the time evolution of the adsorption process. The present paper aims to cover the existing gap using the thermodynamic framework combined with the diffusion-based description of adsorbate time evolution inside an adsorbent. We obtained self-consistent equations describing equilibrium and out-of-equilibrium adsorption, as well as deformation processes. Further, the obtained equations were verified on the experimental data of carbon dioxide and methane on activated carbons. The model is capable of describing both equilibrium and kinetic adsorption and adsorption-induced deformation data. Additionally, we studied the possible influence of slow relaxation processes in the adsorbent on the adsorption process. The current work helps to interpret experimental data for time-dependent adsorption-induced deformation.

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Kinetics of Adsorption-Induced Deformation of Microporous Carbons

Kolesnikov,

Shkolin,

Men’shchikov

et al. 2024

Langmuir

View full text Add to dashboard Cite

show abstract

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Measuring Mass Transfer of n-Hexane and 2-Chloroethyl Ethyl Sulfide in Sorbent/Polymer Fiber Composites Using a Volumetric Adsorption Apparatus

Cited by 1 publication

References 67 publications

Kinetics of Adsorption-Induced Deformation of Microporous Carbons

Kinetics of Adsorption-Induced Deformation of Microporous Carbons

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